namespace CrMap.Models
{
    public class Symbol
    {
        public char Character { set; get; }
        public string CharacterCode { set; get; }
    }
}

using System;
using System.Collections.Generic;
using System.Windows.Media;
using CrMap.Models;

namespace CrMap.ViewModels
{
    public class CrMapViewModel
    {
        public IList<Symbol> Symbols { set; get; }
        public int GridRows { set; get; }
        public int GridCols { set; get; }

        public CrMapViewModel()
        {
            fillDataSource();
        }

        private void fillDataSource()
        {
            Symbols = new List<Symbol>();
            GridCols = 15;

            var fontFamily = new FontFamily(new Uri("pack://application:,,,/"), "/Fonts/#whhglyphs");

            GlyphTypeface glyph = null;
            foreach (var typeface in fontFamily.GetTypefaces())
            {
                if (typeface.TryGetGlyphTypeface(out glyph) && (glyph != null))
                    break;
            }

            if (glyph == null)
                throw new InvalidOperationException("Couldn't find a GlyphTypeface.");

            GridRows = (glyph.CharacterToGlyphMap.Count / GridCols) + 1;

            foreach (var item in glyph.CharacterToGlyphMap)
            {
                var index = item.Key;
                Symbols.Add(new Symbol
                {
                    Character = Convert.ToChar(index),
                    CharacterCode = string.Format("&#x{0:X}", index)
                });
            }
        }
    }
}

<Window x:Class="CrMap.MainWindow"
        xmlns="http://schemas.microsoft.com/winfx/2006/xaml/presentation"
        xmlns:x="http://schemas.microsoft.com/winfx/2006/xaml"
        xmlns:vm="clr-namespace:CrMap.ViewModels"
        Title="MainWindow" WindowStartupLocation="CenterScreen" WindowState="Maximized"
        Height="350" Width="525">
    <Window.Resources>
        <vm:CrMapViewModel x:Key="vmCrMapViewModel" />
    </Window.Resources>
    <ScrollViewer VerticalScrollBarVisibility="Visible">
        <ItemsControl
                      DataContext="{StaticResource vmCrMapViewModel}"  
                      ItemsSource="{Binding Symbols}"
                      Name="MainItemsControl"
                      VerticalAlignment="Top"     
                      HorizontalAlignment="Center"
                      Grid.Column="0" Grid.Row="1" Grid.ColumnSpan="4">
            <ItemsControl.ItemsPanel>
                <ItemsPanelTemplate>
                    <UniformGrid
                        HorizontalAlignment="Center"
                        VerticalAlignment="Center"
                        Columns="{Binding GridCols}" 
                        Rows="{Binding GridRows}">
                    </UniformGrid>
                </ItemsPanelTemplate>
            </ItemsControl.ItemsPanel>
            <ItemsControl.ItemTemplate>
                <DataTemplate>
                    <ContentControl>
                        <Border BorderBrush="SlateGray"
                            HorizontalAlignment="Stretch" VerticalAlignment="Stretch"
                            BorderThickness="1" CornerRadius="3" Margin="3">
                            <StackPanel Margin="3" Orientation="Vertical">
                                <TextBlock                                         
                                    HorizontalAlignment="Center" 
                                    VerticalAlignment="Center" 
                                    FontFamily="Fonts/#whhglyphs"
                                    Foreground="DarkRed"
                                    FontSize="17"
                                    Text="{Binding Character}" />
                                <TextBlock                                         
                                    HorizontalAlignment="Center" 
                                    VerticalAlignment="Center" 
                                    Text="{Binding CharacterCode}" />
                            </StackPanel>
                        </Border>
                    </ContentControl>
                </DataTemplate>
            </ItemsControl.ItemTemplate>
        </ItemsControl>
    </ScrollViewer>
</Window>